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When you see the cutscene where they point guns at eachother, run upstairs and outside the right door immediately to find Pius getting away.
If you want to cut Pius off completely, go around the left side of the castle and shoot out the boards that act as a walkway along the castle balconies. Pius will stay put and wait for you to come get him (you'll still have to intimidate and stun him though).
The other guy, Castrioti is easy to get - once you see the cutscene, he's immediately upstairs and to the left packing - just throw a flashbang at him or something.
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